The crystal formation of CVD—ZnS can be divided into two phases: the nucleation and growth of the fine grains with equiaxial shape on the substrate surface, and then the growth of the coarse columnar grains on the fine grain layer.

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The microstructure of supercooling solidification is made up by four characteristic regions, from the sample bottom to top are: fine equiaxial dendrites, transition from fine equiaxial dendrites to columnar dendrites, columnar dendrites and coarse equiaxial dendrites.

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